Didin Agustian Permadi et al. Correspondence to: Nguyen Thi Kim Oanh

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1 Supplement of Atmos. Chem. Phys., 8, , 28 Author(s) 28. This work is distributed under the Creative Commons Attribution 3. License. Supplement of Integrated emission inventory and modeling to assess distribution of particulate matter mass and black carbon composition in Southeast Asia Didin Agustian Permadi et al. Correspondence to: guyen Thi Kim Oanh The copyright of individual parts of the supplement might differ from the CC BY 3. License.

2 Supplementary Information (SI) Table S. Definition of statistical measures used for WRF/CHIMERE output evaluation. Parameters Formula Suggested criteria Mean bias (MB) WS :.5 m s MB M i O i - WD : deg i T :.5 o C H : g kg - Mean absolute gross error WD : + deg (MAGE) MAGE M i O i T : +2 o C i H : +2 g kg - Root mean squared error WS : +2 m s - (RMSE) 2 RMSE M i O i i Mean fractional bias(mfb) 2 2 M i Oi MFB M O Mean fractional error (MFE) 2 2 MFE M M i i i i O i O i.. PM criteria : ± % PM criteria : +75 % otes: Adapted from the compilation by Kim Oanh et al. (22) M-modeled value (model outputs for the first layer in different grids); O-observations; -number of observations; WS-Wind Speed; WD-Wind Direction; T-Temperature; H- Relative Humidity. Sources: Emery et al. (2), 2 Boylan and Russell (2).

3 Table S2. Summary of ground observations used for model evaluation. o Data sources Data type Information ame longitude latitude Meteorological parameters Olongapo-Phillippines TMP, RH, DIR, SPD RPLB Davao-Phillippines TMP, RH, DIR, SPD RPMD Don Muang-Thailand TMP, RH, DIR, SPD VTBD Trat-Thailand TMP, RH, DIR, SPD VTBO Pnom Penh-Cambodia TMP, RH, DIR, SPD VDPP Jakarta-Indonesia TMP, RH, DIR, SPD WIII Kuala Lumpur-Malaysia TMP, RH, DIR, SPD WMKK Sarawak-Malaysia TMP, RH, DIR, SPD WBKK Ground measurement of aerosols AIRPET project Daily (24h) average of PM, PM 2.5, BC, and OC ambient concentrations 2 AP project Hourly EC/BC and OC 4 Urban air quality Hourly PM monitoring network in Bangkok, Thailand 5 Urban air quality monitoring network in Kuala Lumpur, Malaysia City air quality monitoring network in Surabaya, Indonesia Hourly PM Hourly PM AIT, Thailand (suburban) Tegallega (TL), Indonesia (mix urban) Manila (MO), Philippines observatory (mix urban) Thuong Dinh (TD), Vietnam (mix urban) AIT, Thailand (suburban) Klongjun (T), Thailand (mix urban) Huaykwang (T), Thailand (mix urban) Petaling Jaya, Malaysia (Urban) Jerantut, Malaysia(remote) Taman Prestasi (SUF) Indonesia (mix urban) Ground measurement of AOD AEROET Thailand AOD level 2 Phimai AEROET Singapore AOD level 2 Singapore AEROET Vietnam AOD level 2 Bac Giang AEROET Vietnam AOD level 2 Bac Lieu AEROET Taiwan AOD level 2 Chen Kung AEROET Hong Kong AOD level 2 Hok Sui AEROET Thailand AOD level 2 Mukdahan AEROET Indonesia AOD level 2 Puspitek Serpong..3 9 AEROET Thailand AOD level 2 Silpakorn University. 3.8 AEROET Thailand AOD level 2 Songkhla Met Station. 7.2

4 Table S3. Summary of simulated domain maximum ground-level concentrations PM, PM2.5 and BC for different periods. Pollutants PM (µg m -3 ) PM 2.5 (µg m -3 ) Averaging period a Month, 27 Jan Feb Mar Apr May Jun Jul Aug Sept Oct ov Dec Max hourly Max monthly avg Max annual avg 5 Max hourly Max annual avg Annual average 32 Max hourly BC (µg m -3 ) Max monthly avg Max annual avg ote: a One maximum value simulated in the whole modeling domain for the considered period.

5 Figure S. Modeling domains of WRF and CHIMERE.

6 CH₄ CO/ MVOC OC BC ₂O PM₂. PM₁ H₃ Ox SO₂ CH₄/ CO/ MVOC OC BC ₂O PM₂. PM₁ H₃ Ox SO₂ CH₄ CO/ MVOC OC BC ₂O PM₂. PM₁ H₃ Ox SO₂ Indonesia, BY Cambodia, BY Thailand, BY Emission (Gg yr - ) Energy industry Transportation Fugitive emission Crop residue Solid waste Manufacturing industry Residential and commercial combustion Industrial processes Forest fire Other Figure S2. Total emission and shares for Indonesia, Cambodia and Thailand for base year of 27.

7 Temperature Temperature ( C) Kuala lumpur-malaysia Pnom Penh-Cambodia Wind speed (m/s) Wind speed (m/s) Kuala lumpur-malaysia Pnom Penh-Cambodia Relative humidity (%) Relative humidity (%) Kuala lumpur-malaysia Pnom Penh-Cambodia Temperature ( C) Jakarta-Indonesia Wind speed (m/s) Jakarta-Indonesia Relative humidity (%) Jakarta-Indonesia Figure S3a. Time series of daily average modeled (WRF) vs. observed relative humidity, temperature and wind speed at three WMO stations in Kuala Lumpur (Malaysia), Phnom Penh (Cambodia), and Jakarta (Indonesia) for period of January March 27.

8 Temperature Temperature ( C) Temperature Pnom Penh-Cambodia Kuala lumpur-malaysia Jakarta-Indonesia Wind speed (m/s) Wind speed (m/s) Wind speed (m/s) Kuala lumpur-malaysia Pnom Penh-Cambodia Jakarta-Indonesia Relative humidity (%) Relative humidity (%) Relative humidity (%) Kuala lumpur-malaysia Jakarta-Indonesia Pnom Penh-Cambodia Figure S3b. Time series of daily average modeled (WRF) vs. observed relative humidity, temperature and wind speed at three WMO stations in Kuala Lumpur (Malaysia), Phnom Penh (Cambodia), and Jakarta (Indonesia) for period of August October 27.

9 WRF, Jan ERA interim, Jan WRF, Oct 8 ERA interim, Oct 8 WRF, ov 7 ERA interim, ov 7 Figure S4. Comparison of modeled surface pressure and ERA interim reanalysis data for the selected days in 27 at : UTC.

10 WRF, Jan ERA interim, Jan WRF, Oct 8 ERA interim, Oct 8 WRF, ov 7 ERA interim, ov 7 m s - Figure S5. Comparison of modeled and ERA upper wind fields at 85 hpa on the selected days in 27 at : UTC.

11 4 PBL (m) 2 January February March April May June Month July August September October ovember December Figure S. Domain maximum hourly values of simulated PBL for the different months.

12 PM PM 2.5 BC Figure S7. Simulated annual average of PM, PM2.5 and BC concentrations of 27 over the domain.

13 a) PM, 22 Jan b) PM, 2 ov c) Wind field ( m), 22 Jan d) Wind field ( m), 2 ov e) Hourly precipitation, 22 Jan f) Hourly precipitation, 2 ov Figure S8. Typical simulated maximum hourly PM concentration and wind field at m in 22 January and 2 ovember, : UTC.

14 BC AOD, January BC AOD, August BC AOD BC AOD, ovember BC AOD, December BC AOD ovember Figure S9. Monthly average of simulated BC AOD for the selected months.

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