Trans-boundary Ozone Pollution. A Global Chemical and Aerosol Data Assimilation Perspective. Brad Pierce NOAA/NESDIS
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1 Trans-boundary Ozone Pollution A Global Chemical and Aerosol Data Assimilation Perspective Brad Pierce NOAA/NESDIS
2 Satellite Data Used in RAQMS Ozone Analysis
3 The Ozone Monitoring Instrument (OMI) measures the radiation backscattered by the Earth s atmosphere and surface in the wavelength range nm. Total column O3 error is generally less than 2%. Pixel size is 13x24km. O3 Absorption Spectrum at OMI Wavelengths Radiance Contribution Functions Balis, D., et al. (2007), Validation of Ozone Monitoring Instrument total ozone column measurements using Brewer and Dobson spectrophotometer ground-based observations, J. Geophys. Res., 112, D24S46, doi: /2007jd
4 The Microwave Limb Sounder (MLS) MLS measures millimeter and sub-millimeter emission by scanning the Earth s atmospheric limb. Accuracy of MLS ozone profile is about 8% or better. Provides profile retrievals every 165km along the suborbital track. Band 7 (240 GHz) radiances vs altitude A=primary ozone emission line MLS Averaging Kernels Froidevaux, L., et al. (2008), Validation of Aura Microwave Limb Sounder stratospheric ozone measurements, J. Geophys. Res., 113, D15S20, doi: /2007jd
5 RAQMS O3 Assimilation Procedure OMI cloud cleared O3 column Demonstration of: Real-time assimilation of Microwave Limb Sounder (MLS) stratospheric ozone profiles Real-time assimilation of Ozone Monitoring Instrument (OMI) total ozone column Real-time incorporation of Moderate Resolution Imaging Spectroradiometer (MODIS) fire detection
6 Contribution of Asian Wildfires to Intercontinental Pollution Transport (April 2008 ARCTAS/ARCPAC Campaigns)
7 RAQMS OMI+MLS Ozonesonde Validation April 2008 April 2008 RAQMS vs ARCIONS ozonesonde (182 North American sondes) +/-20% ANNE M. THOMPSON SAMUEL OLTMANS DAVID TARASICK
8 Dupont, R. et al., Reconstructing ozone chemistry from Asian wild fires using models, satellite and aircraft measurements during the ARCTAS campaign, Atmos. Chem. Phys. Discuss., 10, , 2010, doi: /acpd NASA DC8 Flight Track 04/19/2008 DIAL 591 nm Aerosol Scattering Ratio DIAL aerosol measurements: John Hair, NASA/LaRC
9 Trinidad Aeronet vs RAQMS AOD: April 2008 April 22 nd,2008 Biomass burning aerosols observed at Trinidad Head on April 22, 2008 RAQMS analysis overestimates AOD associated with biomass burning plume relative to Aeronet
10 Impacts of Kazakhstan/Baykal/Thailand wildfires O3 Column 400mb-SFC Delta-O3 Cross-section Delta-O3 Column 400mb-SFC 120W Impact of Kazakhstan/Baykal/Thailand wildfires on tropospheric ozone production extends into North America with potential US Air Quality impacts Natarajan, M., et al. (2012), Radiative forcing due to enhancements in tropospheric ozone and carbonaceous aerosols caused by Asian fires during spring 2008, J. Geophys. Res., 117, D06307, doi: /2011jd
11 Contribution from East Asian Emissions to Intercontinental Pollution Transport (May-June 2010 CalNex Campaign)
12 CalNex-2010 O 3 sondes Owen Cooper (NOAA ESRL) CalNex Ozonesonde RAQMS OMI+MLS Ozonesonde Validation May-June /-20%
13 Comparison with NOAA P3 Insitu O3 Measurements (Primarily LA Basin/Central Valley) No Assim MLS+OMI Assim P3 O3 from Tom Ryerson, NOAA/ESRL Assimilation of MLS+OMI O3 retrievals results in increased lower-tropospheric O3 (and improved agreement with airborne insitu O3) over Southern California
14 Impacts of East Asian Emissions May 2010 O3 Column 400mb-SFC Delta-O3 Cross-section Delta-O3 Column 400mb-SFC 120W Impact of East Asian ozone production extends into North America with potential US Air Quality impacts The Task Force on Hemispheric Transport of Air Pollution (TF HTAP) is an international scientific cooperative effort to improve the understanding of the intercontinental transport of air pollution across the Northern Hemisphere.
15 Impacts of East Asian Emissions May 2010 CO Column 400mb-SFC Delta-CO Cross-section Delta-CO Column 400mb-SFC 120W Impact of East Asian ozone production extends into North America with potential US Air Quality impacts The Task Force on Hemispheric Transport of Air Pollution (TF HTAP) is an international scientific cooperative effort to improve the understanding of the intercontinental transport of air pollution across the Northern Hemisphere.
16 distribution of O3/CO mixing ratios (135W-125W) Total, and Pollution (O3>60ppbv, CO>150ppbv) contributions
17 135W-125W Zonal Mean O3 March-July Mean O3 >60ppbv extends below 3km at 25N 135W-125W Zonal Mean CO March-July Mean CO shows significant NS gradient above O3>60ppbv isopeth mixing of stratospheric (high O3/low CO) air
18 135W-125W Zonal Mean Pollution O3 March-July Mean Pollution O3 >15ppbv Pollution (O3>60ppbv,CO>150ppbv)) 135W-125W Zonal Mean Pollution CO March-July Mean Pollution CO >40ppbv
19 135W-125W Zonal Mean Pollution O3 (ppbv) March Pollution (O3>60ppbv,CO>150ppbv) 135W-125W Zonal Mean Pollution CO (ppbv) March March: polluted O3 (30ppbv) and CO (80ppbv) mean mixing ratios Note: 2x change in color scale
20 135W-125W Zonal Mean Pollution O3 (ppbv) April Pollution (O3>60ppbv,CO>150ppbv) 135W-125W Zonal Mean Pollution CO (ppbv) April April: polluted O3 (>40ppbv) and CO (>80ppbv) mean mixing ratios
21 135W-125W Zonal Mean Pollution O3 (ppbv) May Pollution (O3>60ppbv,CO>150ppbv) 135W-125W Zonal Mean Pollution CO (ppbv) May May: polluted O3 (25ppbv) and CO (50ppbv) mean mixing ratios
22 135W-125W Zonal Mean Pollution O3 (ppbv) June Pollution (O3>60ppbv,CO>150ppbv) 135W-125W Zonal Mean Pollution CO (ppbv) June June: polluted O3 (<10ppbv) and CO (<20ppbv) mean mixing ratios
23 135W-125W Zonal Mean Pollution O3 (ppbv) July Pollution (O3>60ppbv,CO>150ppbv) 135W-125W Zonal Mean Pollution CO (ppbv) July July: polluted O3 (10ppbv) and CO (20ppbv) mean mixing ratios
24 Spring 2015 Intercontinental Pollution Transport Event (March 22-24, 2015)
25 ??
26 Reverse Domain Filling (RDF) Analysis Re-map to Day=0 grid Day=-5 Average along backtrajectory Day=0 Pierce, R. B. et. al. (2009), Impacts of background ozone production on Houston and Dallas, TX Air Quality during the TexAQS field mission, J. Geophys. Res., 114, D00F09, doi: /2008jd011337
27 Lagrangian Averaged O3 3km AGL 5 Day RDF Analysis 18Z 03/22/2015 Lagrangian Averaged CO Lagrangian Averaged O3 P-L East Asian PBL Exposure
28 Lagrangian Averaged O3 3km AGL 5 Day RDF Analysis 18Z 03/23/2015 Lagrangian Averaged CO Lagrangian Averaged O3 P-L East Asian PBL Exposure
29 Lagrangian Averaged O3 3km AGL 5 Day RDF Analysis 18Z 03/24/2015 Lagrangian Averaged CO Lagrangian Averaged O3 P-L East Asian PBL Exposure
30 Summary: Global assimilation of MLS stratospheric O3 and OMI cloud cleared total column O3 results in well constrained ozone analyses over North America but upper tropospheric ozone variability is still underestimated Ozone production from SE Asian fires and industrial emissions have similar magnitude impacts (6-8ppbv) on ozone off the west coast of the US during the Spring (April/May) RAQMS O3 analyses show that, on average, the mean polluted (O3>60ppbv/CO>150ppbv) Eastern Pacific air masses have O3 mixing ratios that reach peaks in excess of 40ppbv in April but decline significantly (<10ppbv) in June Reverse Domain Filling techniques can be used to identify the origins and net photochemical ozone production during intercontinental pollution events
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