Testing of the Toyota Avensis DPNR at U.S. EPA-NVFEL SAE TECHNICAL PAPER SERIES

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SAE TECHNICAL PAPER SERIES 2002-01-2877 Testing of the Toyota Avensis DPNR at U.S. EPA-NVFEL Joseph McDonald and Byron Bunker U.S. EPA Office of Transportation and Air Quality and Powertrain and Fluid Systems Conference & Exposition San Diego, California, USA October 21-24, 2002 400 Commonwealth Drive, Warrendale, PA 15096-0001 U.S.A. Tel: (724) 776-4841 Fax: (724) 776-5760

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2002-01-2877 Testing of the Toyota Avensis DPNR at U.S. EPA-NVFEL Joseph McDonald and Byron Bunker U.S. EPA Office of Transportation and Air Quality ABSTRACT An advanced prototype of the Toyota Avensis light-duty diesel vehicle equipped with a version of Toyota s DPNR exhaust emission control system was tested at the U.S. EPA NVFEL facility. The vehicle is under development by Toyota Motor Corporation for introduction in Europe. While this particular model is not anticipated to be offered for sale in the U.S., EPA evaluated the vehicle to gauge the current state of light-duty diesel vehicle technology. The vehicle was tested using a low sulfur (6 ppm) diesel fuel with a cetane number that was improved to near typical European levels (~50 cetane). Emission levels over the FTP75 consistent with U.S. Federal Light-Duty Tier 2 emission standards were achieved at levels of fuel economy that are competitive with current light-duty diesel passenger vehicles offered for sale in the U.S. The vehicle was tested with relatively low accumulated mileage. Further testing at 50,000-120,000 accumulated miles will be necessary to determine the long-term durability of the emission control system. INTRODUCTION The Office of Transportation and Air Quality (OTAQ) of the U.S. Environmental Protection Agency (U.S. EPA) is currently evaluating progress in the development and application of NOx exhaust emission control systems for heavy-duty diesel trucks, buses, and light-duty diesel vehicles. This evaluation will gauge progress towards meeting new U.S. Federal Heavy-duty Engine emissions standards for heavy-duty buses and trucks that will phase-in beginning with model year 2007. It will also provide information to EPA on progress being made to introduce clean, fuel-efficient diesel technology that can be certified to meet the new U.S. Federal Light-duty Tier 2 emission standards that will phase-in for passenger vehicles between the 2004 and 2007 model years. This report summarizes testing conducted on a mid-size lightduty diesel passenger vehicle incorporating recently developed technology to control NOx and PM emissions to very low levels. The vehicle was provided by Toyota Motor Corporation. The Toyota Avensis Diesel is currently under development for the European market with a target of having lower emissions than the European Stage IV emission levels. This vehicle is not intended for sale in the U.S., and has not been specifically developed to meet current or future U.S. vehicle emission standards. TEST PROCEDURES VEHICLE DESCRIPTION The vehicle tested was a new version of the Toyota Avensis mid-size light-duty passenger vehicle marketed by Toyota in Europe. Major vehicle specifications are summarized in Table 1. The vehicle is equipped with a turbocharged, direct-injection diesel engine. The new Toyota Avensis diesel engine uses an electronically controlled high-pressure common-rail fuel system, highpressure-loop electronically controlled EGR, and an electronically controlled intake throttle. Under some light-load conditions, the engine operates using a smokeless low-temperature combustion mode developed by Toyota Motor Corporation 1. The Toyota Avensis was also equipped with Toyota s Diesel Particulate NOx Reduction (DPNR) system 2. This system incorporates a NOx adsorber catalyst and a catalyzed diesel particulate filter within a single catalyzed wall-flow monolith. Toyota has previously demonstrated NOx and PM emissions reductions of greater than 80% for this type of exhaust emission control system. The vehicle was also equipped with a diesel oxidation catalyst (DOC) for additional control of hydrocarbon and CO emissions. The vehicle provided by Toyota was a pre-production engineering prototype with relatively low accumulated mileage. As such, emissions performance should be considered to be for a relatively unaged catalyst and emission control system. The vehicle tested is similar to the 60 vehicles that will participate in an 18-month monitoring program in Europe during 2002-2003 3.

Table 1: Summary of major vehicle specifications. Manufacturer/Model: Prototype Toyota Avensis DPNR Vehicle Type: Small station wagon Interior Passenger and Cargo Volume: 3.62 m 3 Power Transmission: Front-drive, 5-speed manual transmission Engine: 2.0 L, 4-cyl. Turbocharged, charge-air-cooled DI Diesel w/dohc and 4 valves/cyl. Power/Torque Rating: 81 kw @ 4000 rpm 250 Nm @ 2000 rpm Fuel System: Denso HPCR Emission Control Systems: DPNR system, cooled EGR, Catalyst Volume: DPNR: 2.8 L DOC: 2.0 L Inertia Weight (as tested): 1590 kg Table 2: Summary of fuel properties. Test Method Results Net Heat of Combustion, ASTM D3338-92 (MJ/kg) 43.11 Density @ 15.5 ºC (g/cm 3 ) 0.891 Cetane Number 50.2 Cetane Index 51.7 Olefins, FIA D1319-93 (% Vol.) 2.7 Aromatics, D1319-93 (% Vol.) 27.5 Sulfur, ASTM D2622 (ppm mass) 9 Carbon, ASTM D3343-95 (% mass) 0.8654 Distillation Properties, ASTM D86 IBP (ºC): 189 10 % (ºC): 218 50 % (ºC): 260 90 % (ºC): 316 End Point (ºC): 347 Residue Diesel (%): 1.0 Recovery: 99.9% Note: Fuel additive (2-ethyl-hexyl-nitrate) used to raise cetane number from ~43 to ~50. Table 3: Exhaust gas analyzers. Bag-sample Dilute Gas Analyzers Species Horiba AIA-23 NDIR CO Horiba AIA-23 NDIR CO 2 Beckman 400 FID Beckman 951A CLD NOx Continuos Dilute Gas Analyzers Horiba FIA-220 HFID THC Rosemount 955 HCLD NOx TEST FUEL The fuel used for all testing was Phillips Chemical Company Lot 1APULD02. This fuel was similar to that specified by the U.S. Department of Energy s Diesel Emission Control-Sulfur Effects (DECSE) program to have properties comparable to today s on-highway fuel with the exception of very low sulfur content. The engine was originally calibrated for use with diesel fuels available in Western Europe. Approximately 0.1% by mass of a common cetane additive (Ethyl Corporation, HiTEC 4103 Cetane Improver) was added to the fuel. The cetane additive (chiefly 2-ethylhexyl nitrate) was added to raise cetane number from 43 to 50 in order to provide compression ignition properties closer to that of fuels for which the engine was originally calibrated. The properties of the fuel used are summarized in Table 2. TEST CYCLES Examples of the driving traces used for chassis dynamometer testing are presented in the appendix. The vehicle was tested using the full range of chassis dynamometer test cycles required for Tier 2 certification. This included the FTP75, US06, SC03, and highway fuel economy driving cycles. The environmental conditions of the SCO3 test were simulated using a modified version of the AC2 test procedure 4. The modifications to the AC2 procedure included operation at ambient conditions of 35 ºC ± 1 ºC with the vehicle windows down and the air-conditioner at its lowest temperature setting. The vehicle was also tested using the New York City Cycle to simulate operation in heavily congested urban areas. FACILIITIES Testing was conducted at the U.S. EPA National Vehicle and Fuel Emission Laboratory (NVFEL) in Ann Arbor, MI USA. The vehicle was tested using a 48 -diameter single-roll, electric chassis dynamometer. A summary of track and dynamometer coast-down data, including the derived dynamometer coefficients, is included in the Appendix. Vehicle exhaust was diluted using a full-flow, low-particle-loss dilution system developed by EPA. A description of the features of this system is included in the appendix. A PHILCO CFV-CVS was used for flow control of the dilute exhaust, and was operated at a nominal flow-rate of 750 scfm. Table 3 contains a summary of the exhaust gas analytical equipment used.

RESULTS Emissions and fuel economy results are summarized in Table 4. PM emissions over the FTP75 drive cycle were at approximately one-half of the Tier 2 standards for certification bins 2 through 6. The NOx and NMHC emissions were at or just under the Tier 2 bin 5 50,000 mile FTP emission standards. Approximately 75% of the emissions during phase-1 of the FTP75 were from the second of the five accelerations following the cold-start (figure 1). Immediately after the second acceleration, minimal additional NOx was accumulated over phase-1. NOx emissions over phase-2 of the FTP75 were essentially zero. During phase-3 of the FTP75, the accumulated mass of NOx emissions was only ~10% of the mass accumulated over phase-1. As with phase-1, a majority of the NOx emissions accumulated over phase-3 of the FTP75 were associated with the second acceleration following the hot-start. NOx accumulated as a series of break-through events that occurred primarily over the first half of the US06 (figure 2). NOx emissions were at or below background levels over the SC03, HWFET, and NYCC drive cycles. NMHC emissions were roughly comparable over phase- 1 and phase-3 of the FTP75 test. Emission levels of NMHC for the hot-stabilized (phase 2) portion of the FTP were approximately half that of phases 1 and 3. Hydrocarbon mass-emissions appeared to accumulate at near-constant rates over each phase of the FTP75 (figure 1) and over the over the US06 (figure 2), SC03, and HWFET drive cycles. It is possible that NMHCcontrol with this vehicle would benefit from additional oxidation catalyst volume or activity. The measured mass emissions from the continuous heated FID measurement had coefficients of variance of approximately 20 to 50% over the range of drive cycles. This was likely due to the very low level of measured NMHC emission. Additional testing using more sensitive HFID instrumentation would be necessary to draw further conclusions with respect to NMHC emissions from this vehicle at such low emission levels. NOx and HC emissions from the Toyota Avensis DPNR over phase-1 of the FTP75 test are compared to those of a similar gasoline vehicle certified to California LEV-I LEV standards in figure 3. Stabile control of NOx emissions occurred later for the Toyota Avensis DPNR, indicating a somewhat longer period prior to NOx storage and/or light-off compared to the time to light-off for a conventional 3-way LEV catalyst system. NOx emissions, however, were considerably less for the Toyota Avensis DPNR in the period prior to achieving the NOx light-off temperature, which would indicate lower engine-out NOx emissions than the gasoline LEV vehicle immediately following the cold-start or some low temperature NOx storage depending on the engine-out level of NO 2 present in the exhaust at such relatively low exhaust temperatures. The Toyota Avensis DPNR demonstrated improved fuel economy when compared to the highest fuel economy conventional gasoline vehicles sold in the U.S. for the 2002 model year (table 6). Fuel economy was less than the highest fuel economy diesel vehicle currently offered for sale in the U.S., the 2002 VW Jetta Wagon. It should be noted that the VW Jetta Wagon is a lighter vehicle. The Jetta was also certified to U.S. Federal Tier 1 diesel emission standards that represent PM and NOx emission levels that are approximately an order of magnitude higher than the levels measured from the Toyota Avensis DPNR. Table 4: Summary of exhaust emission and fuel economy results Test PM NOx NMHC CO CO 2 FE Cycle (mg/mi) (g/mi) (g/mi) (g/mi) (g/mi) (mi/gal) Tier 2 10 0.05 0.075 3.4 bin 5 Tier 2 10 0.08 0.075 3.4 bin 6 FTP75 5.7 0.05 0.07 0 273 37.2 (± 0.8) (± 0.01) (± 0.03) (± 2) (± 0.2) US06 5 0.14 0.19 0 289 35.2 (± 3) (±.0.04) (± 0.07) (± 7) (±0.8) SC03 7 (±2) 0 0.14 (± 0.09) 0 367 (± 3) 27.7 (± 0.3) HWFET 2 (± 1) 0 0.12 (±0.07) 0 192 (± 2) 52.9 (0.7) NYCC 7 (±2) 0 0.04 (± 0.01) 0 474 (±10) 21.5 (± 0.5) Notes: 50,000 mile Tier 2 bin 5 and bin 6 emission standards shown for comparison purposes. A summary of Tier 2 standards can be found in Appendix Table 1. The ± values represent 95% confidence intervals for a two-sided students t-test with 3 to 4 FTP75, US06,SC03, and HWFET replicates; and 6 NYCC replicates. Bag-sampled results are shown for NOx, CO, and CO 2. NMHC was derived from integrated-continuous heated- FID measurements and bag-sampled CH 4. Fuel economy results are reported here as unadjusted test results. Table 5: Comparison of Toyota Avensis DPNR emissions results to 4,000 mile light-duty Tier 2 SFTP emission standards US06 SC03 NMHC+ CO NMHC+ CO NOX (g/mi) NOX (g/mi) (g/mi) (g/mi) Tier 2 SFTP Standard (4k miles) 0.14 8.0 0.20 2.7 Toyota Avensis DPNR 0.33 0 0.14 0

(a) FTP75 Phase 1 (cold start) (b) FTP75 Phase 2 (stabilized) (c) FTP75 Phase 3 (hot start) Figure 1: Accumulation of NOx and THC mass emissions over the 3-phases (cold-start, stabilized, hot-start) of the FTP75 chassis dynamometer drive cycle. Phase 1 cold start emissions (a) were compared to an SIequipped vehicle of comparable size and power that was certified to California LEV standards.

Figure 2: Accumulation of NOx and THC mass emissions over the US06 high-speed chassis dynamometer drive cycle. Figure 3: Phase 1 cold start emissions compared to an SI-equipped vehicle of comparable size and power and certified to California LEV standards.

Table 6: Measured fuel economy of the Toyota Avensis DPNR station wagon to similar vehicles offered for sale in the U.S. Vehicle Type Engine Transmission/ Drive City/Highway Fuel Economy (mi/gal) Toyota Avensis Small Station 2.0-L 4-cyl. Turbo-Diesel 5-speed Manual/ DPNR Wagon with charge-air cooling Front-drive 2002 VW Jetta Small Station 1.9-L 4-cyl. Turbo-Diesel 5-speed Manual/ Wagon 2002 Ford Focus Station Wagon Wagon Mid-size Station Wagon with charge-air cooling 2.0-L NA SI gasoline Front-drive 5-speed Manual/ Front-drive Test Weight (lbs.) 33/41 3500 42/50 3375 28/36 3125 2002 Honda Mid-size Passenger 2.3-L NA SI gasoline 5-speed Manual/ 26/32 3250 Accord Vehicle Front-drive Notes: The 2002 VW Jetta Wagon, Ford Focus Station Wagon, and Honda Accord included in this comparison demonstrated the highest combined fuel economy for their respective vehicle classes. Fuel economy results for Toyota Avensis include adjustments of 10% over the city cycle and 22% over the highway cycle to better suit realworld driving conditions and to allow comparison with values reported in the Fuel Economy Guide. CONCLUSION The Toyota Avensis DPNR demonstrated emissions over the FTP75 drive cycle that were consistent with a vehicle capable of meeting the mid- to upper-bins (bins 5-8) of the Tier 2 emissions standards. With moderate improvements in HC emissions, the Toyota Avensis vehicle would be capable of achieving Tier 2 bin 5 or bin 6 emissions over the FTP75 using low sulfur diesel fuel similar to fuels that will be available in the U.S. after 2006 if the emission control system is relatively durable up to the statutory full useful life (120,000). Further NOx and NMHC reductions over the US06 drive cycle should be necessary for a vehicle of this type to meet Tier 2 SFTP standards. ACKNOWLEDGMENTS The authors wish to thank the Toyota Motor Corporation and the Toyota Technical Center for their provision of an advanced prototype vehicle for testing by EPA, especially Dr. Kiyoshi Nakanishi, Dr. Koichiro Nakatani, Mr. Taro Aoyama, Mr. Tadao Shimbori and Mr. Thomas Beiershmitt. The authors also would like to thank the engineers and technicians of the Laboratory Operations Division at the U.S. EPA-NVFEL facility in Ann Arbor, MI, especially Mr. David Bochenek and Mr. John Menter. REFERENCES 1. S. Sasaki, T. Ito, S. Iguchi, Rußarme fette Verbrennung mit Niedertemperatur-Oxydation in Diesel Motoren, 9. Aachener Kolloquium Fahrzeugund Motorentechnik 2000 ( Smoke-less Rich Combustion by Low Temperature Oxidation in Diesel Engines, 9 th Aachen Colloquium Automobile and Engine Technology 2000). 2. K. Nakatani, S. Hirota, S. Takeshima, K. Itoh, T. Tanaka, K. Dohmae, Simultaneous PM and NOx Reduction System for Diesel Engines, SAE Technical Paper Series, No. 2002-01-0957. 3. Press release, Toyota Motor Corporation, March 6, 2002 (Internet URL: http://global.toyota.com/ci.html) 4. U.S. Code of Federal Regulations, Part 86, Subpart B, section 86.162, 2000. APPENDIX Appendix Table 1: Summary of U.S. Federal Tier 2 Light-Duty Vehicle and Truck Intermediate-Life (50,000 mile) Emission Standards. Bin Number NOx (g/mi) NMOG (g/mi) CO (g/mi) HCHO (g/mi) 10 0.4 0.125 3.4 0.015 9 0.2 0.075 3.4 0.015 The above temporary bins expire in 2006 (for LDVs and LLDTs) and 2008 (for HLDTs) 8 0.14 0.100 3.4 0.015 7 0.11 0.075 3.4 0.015 6 0.08 0.075 3.4 0.015 5 0.05 0.075 3.4 0.015

Appendix Table 2: Track coast down-data, dynamometer coast-down data, and derived dynamometer coefficients Speed Expected Actual Time Expected Force Actual Force Range Time (s) (N) (N) (km/hr) (s) 125-115 6.81 6.78 659 662 115-105 7.77 7.77 577 578 105-95 8.92 8.92 503 503 95-85 10.29 10.30 436 436 85-75 11.93 12.01 376 374 75-65 13.88 14.03 323 320 65-55 16.17 16.22 277 277 55-45 18.8 18.86 239 238 45-35 21.67 21.90 207 205 35-25 24.60 27.88 182 180 25-15 27.21 27.83 165 161 15-5 29.07 30.68 154 146 Inertia: 1590 kg Highway Inertia: 1614 kg Dynamometer Coefficient Set points Measured Coefficients A (N) B (N/km/hr) C (N/km/hr ) A (N) B (N/km/hr) C (N/km/hr ) 61.27-0.8526 0.03783 144.31 0.0808 0.03513 Appendix Figure 1: Dynamometer coast-down with vehicle.

Appendix Figure 2: FTP75 Drive Cycle. Appendix Figure 3: Highway Fuel Economy Drive Cycle.

Appendix Figure 4: US06 Drive Cycle. Appendix Figure 5: SC03 Drive Cycle.

Appendix Figure 6: New York City Drive Cycle. Appendix Figure 7: Toyota Avensis DPNR sedan 3. The physical layout of the drivetrain and exhaust emission control system is distinguishable between the sedan and station wagon versions of the Toyota Avensis DPNR.

Appendix Figure 8: Low-particle-loss dilution system. Cyclone and filter packs designed according to 40 CFR 86.1310-2007. Single Pall-Gellman TX- 40 high-efficiency 47mm filters were used for all PM sampling. Filter-face temperature was held to <50 ºC for all reported PM test results. Mixing at the cross-section of the inlet to the sample probes was characterized by tracer gas method as per 40 CFR 86.1310-2007.