AECC/Concawe 2016 GPF RDE PN Test Programme: PN Measurement Above and Below 23nm

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AECC/Concawe 2016 GPF RDE PN Test Programme: PN Measurement Above and Below 23nm Jon Andersson 1, Joachim Demuynck 2, Heather Hamje 3 (1) Ricardo UK; (2) AECC; (3) Concawe June 19th - 22nd, 2017, ETH Zurich, Switzerland

2 Contents Introduction Objectives Measurements Test Cycles Results Conclusions

3 Introduction The introduction of Real Driving Emissions (RDE) and the inclusion of a Particle Number (PN) limit for direct injection gasoline (GDI) vehicles has accelerated the development of Gasoline Particle Filters (GPF) GPFs are expected to appear on mass-market production vehicles during 2017 As part of a larger programme exploring exhaust emissions under RDE, a 1.4 litre Euro 6b stoichiometric lambda 1 GDI was tested in standard build, and when retrofitted with a catalysed-gpf Particle number measurements were made of >23nm PN 23 and >7nm PN 7 size ranges to explore emissions levels and filtration impacts under a range of operating conditions

4 Contents Introduction Objectives Measurements Test Cycles Results Conclusions

5 PN-related Objectives To measure PN emissions from Real Driving Emissions (RDE) tests transposed to a chassis dynamometer and evaluate impact of moving towards RDE boundary conditions, including: Normal and reduced test temperatures: 23 C, 0 C, -7 C Dyno load changes: ~ road load, ~25% increase, ~50% increase To assess the impact of a specific GPF on PN emissions Including impact on PN 7 and PN 23, if different Extras To compare magnitude of PN-PEMS and CVS-based PN emissions To assess any impact of a TWC on PN reduction

6 Contents Introduction Objectives Measurements Test Cycles Results Conclusions

7 PN Systems Sampling Configurations 2 raw systems, 2 dilute systems, >7nm system, 3 x >23nm systems Initial dilution Preclassifier PND 1 (diluter#1) Volatile Removal PND 2 (diluter#2) PNC (counter) 4: Raw PN-PEMS (prototype) 3: Raw SPCS 2: Dilute Catalytic Stripper [-] dilution 10 350 C 1: Dilute SPCS CVS (<30) 1µm dilution 10 <10µm dilution 10 DOC 350 C Evap tube 350 C dilution 10 dilution 15 CVS (<30) [-] [-] [-] <52 C <52 C <10µm dilution 10 ambient ~190 C ~190 C DOC 350 C Evap tube 350 C dilution 15 ambient < 35 C < 35 C d50 23nm d50 23nm d50 7nm* d50 23nm *The emissions levels recorded with the 7nm d50 CPC were corrected for losses in the catalytic stripper

8 Contents Introduction Objectives Measurements Test Cycles Results Conclusions

9 Test Cycles Regulatory Test Cycles at 23 C conducted at dyno load consistent with real road load NEDC WLTC Real Driving Emissions (RDE) Based upon actual valid on-road drive EMROAD processing of RDE using WLTC cycle conducted above On road cycle then transposed to dyno, driven and reprocessed in EMROAD CO 2 levels from on-road and ondyno very close Real Driving Emissions (RDE) performed on dyno with increased acceleration rates Nominated as SRDE (Severitized RDE) Minimal increase in dyno load SRDE_L at 23 C SRDE_L0 at 0 C SRDE_L-7 at -7 C ~25% increase of dyno load SRDE_M ~50% increase of dyno load SRDE_H [also 0 C & -7 C] SRDE variants tested with and without GPF

10 On-dyno RDE EMROAD outputs for On-dyno RDE: SRDE_L, SRDE_M, SRDE_H Average CO 2 mild / Low SRDE_L Average CO 2 moderate / Normal SRDE_M Average Speed Average Speed Average CO 2 severe / High SRDE_H Valid range for RDE data SRDE approach allows the valid RDE space to be explored within the controllable environment of the test laboratory Average Speed

11 Contents Introduction Objectives Measurements Test Cycles Results Conclusions

12 CVS (dilute) and Raw >23nm PN sampling appear sufficiently similar to be considered equivalent Non-GPF sampling Non-GPF sampling Comparison of raw and dilute SPCS systems indicates <5% difference CVS levels are slightly higher May indicate CVS background contribution not present in raw sample Other differences exist though Additional raw diluter Different preclassifier

13 Prototype PN-PEMS system shows good correlation with CVS-based PN 23 system, but ~20% higher levels post-gpf sampling non-gpf sampling Draft RDE regulation requires measured PEMS emissions to be ±50% of CVS levels Easily achieved Higher PEMS-PN levels indicative of differences in: Methodology for corrections of losses Absolute losses (raw v dilute) post-gpf sampling non-gpf sampling Good linearity of relationship allows correction of PN- PEMS data to simulate CVS levels from raw exhaust

14 The Three-Way Catalyst (TWC) is not a major source of particle removal or loss non-gpf sampling Equating non-gpf measurements from the raw SPCS (pre- TWC) with the corrected tailpipe PN-PEMS shows <5% difference non-gpf sampling Losses / elimination of particles in the TWC are <10% With the difference between raw and dilute SPCS factored-in

15 0 C and -7 C SRDE PN 23 data, based upon CVS measurements using dilute SPCS Error bars = 1s of 3 repeats of SRDE_M applied to other tests CF=1.5 Euro 6c/d as the same % Euro 6c/d PN 23 levels rise as cold-start temperature reduces Larger rise 23 C to 0 C than from 0 C to -7 C Post-GPF PN levels rise by ~80% with each step from SRDE_L to SRDE_M to SRDE_H Engine-out PN levels from all conditions equal to, or in excess of CF=1.5 Post-GPF PN 23 levels below CF=1 from all SRDE

PN Emissions >23nm Ricardo plc 2017 16 Relationship between total PN 7 and total PN 23 changes when specific GPF is applied 1.60E+12 1.40E+12 1.20E+12 1.00E+12 8.00E+11 6.00E+11 4.00E+11 2.00E+11 CF=1 Post GPF: PN 7 = ~1.2 x PN 23 Post GPF CF=1 0.00E+00 0.00E+00 6.00E+11 1.20E+12 1.80E+12 2.40E+12 3.00E+12 PN Emissions >7nm NO GPF: PN 7 = >1.5 x PN 23 CVS-based measurements of PN 7 and PN 23 show that all post-gpf tests emissions were below the Euro 6c limit NEDC, WLTC and SRDE_L,M &H testing When a GPF is applied, the differential between the number of particles >7nm and the number of particles >23nm is minimised The GPF appears to preferentially trap the smallest particles Diffusion collection mechanism dominates

17 GPF efficiencies for >23nm particles range from ~60% to ~80%, but are exceeded by >7nm efficiencies (70% to >90%) >7nm >23nm SRDE_L SRDE_M SRDE_H SRDE_H0 SRDE_L-7 SRDE_H-7 Observed increase in filtration efficiency between >7nm and >23nm ranges indicates larger increase for 7nm to 23nm range in isolation (>95%)

18 Contents Introduction Objectives Measurements Test Cycles Results Conclusions

19 Conclusions The addition of a GPF enabled the regulatory limit value for GDI vehicles (6x10 11 #/km) to be achieved, for PN 23, from standard chassis dyno cycles and very demanding RDE conditions, including high load and low temperature tests Increases in engine-out PN of >50% were seen when extending the measurement range from d50=23nm down to ~7nm, but with a GPF in place this differential dropped to ~20% The GPF tested appears especially efficient for <23nm PM CVS (dilute) and Raw PN 23 lab-based PN sampling (the latter currently being considered as an option for certification testing) appear sufficiently similar to be considered equivalent in the configurations used at Ricardo >23nm PN-PEMS particle number emissions proved to be ~20% higher than CVSbased levels, due to lower sampling losses but agreement is well within the ±50% range permitted for regulatory correlation

20 Acknowledgements Thanks to: AECC members Concawe members Staff at Ricardo Simon de Vries Carl Jemma Any questions?