Coupled Neutron-Gamma MultigrouF. Cross Sections for 29 Materials f. to Nuclear Weapons Effect Calc. Generated by LASL/TD Divi: .

c LA-5137 3 -- Coupled Neutron-Gamma MultigrouF Cross Sections for 29 Materials f to Nuclear Weapons Effect Calc Generated by LASL/TD Divi: ( (b ; 10s scientific I I r) of the University < 4 /\, -DO NOT CIRCUL = = alamos laboratory of California LOS ALAMOS, NEW MEXICO 87544 PERMANENT REQUiREDBY RETENTJ( / CONTRA UNITED STATES ATOMIC ENERGY COMMISSION CONTRACT W-7405 -ENG 36

This report was prepared as an account of work sponsored by the United States Government Neither the United States nor the United States Atomic Energy Commissio nor any of their employees, nor any of their contractors, subcontractors, or their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness or usefulness of any informatio apparatus, product or process disclosed, or represents that its use would not infringe privately owned rights Printed in the United States of America Available from National Technical Information Service U S Department of Commerce 5285 Port Royal Road Springfield, Virginia 22151 Price: Printed Copy $76 Microfiche $145 \- i

LA-51 37 UC-34C ISSUED: February 1974 10 scientific Iamos Laboratory of the university of California LOS ALAMOS NEW MEXICO 87544 Coupled Neutron-Gamma Multigroup-Multitable Cross Sections for 29 Materials Pertinent to Nuclear Weapons Effect Calculations Generated by LASL/TD Division by H A Sandmeier G E Hansen R E Seamen T J Hirons A H Marshall A \

COUPLED NSUTRON-GANNA MULTIGROUP-MULTITABLE CROSS SECTIONS FOR 29 MATERIALS PERTINENT TO NUCLEAR WEAPONS EFFECT CALCULATIONS GENERATED BY LASL/TD DIVISION by H A Sandmeier, G E Hanse R E Seame T J Hirons, and A H Marshall ABSTRACT * -J This report lists 42-group, coupled, neutron-ganmnacross sections for H, D, T, 3He, 4He, 6Li, 7Li Be 10B, llb, C, N, O Na, Mg, Al, Si, Cl, A, K, Ca, Fe, CU W, Pb, 23ju, ~38u, 239pua and 24aPU Most of these materials are used in nuclear weapons effects calculations,where the elements for air, ground, and sea water are needed Further, we list C}OSS sections for materials used in nuclear weapons vulnerability calculations, such as the elements ofhigh explosives as well as materials that will undergo fusion and fissio Most of the common reactor materials are also listed, The 42 coupled neutron-gamma groups sre split into 30 neutron groups (17 MeV through 139 x 10-4 ev) and 12 gamma groups (10 MeV through 01 MeV) Data sources and averaging schemes used for the development of these multigroup parameters are give I INTRODUCTIOIT Coupled neutron gamma cross sections are being widely used among vulnerability and weapons effect investigators in the US k!ehave reported their use in several Los Alamos Scientific Laboratory (1ASL)reports dealing with nuclear weapons neutron 1 and gamma output and nuclear weapons effect studies 2 in the atmosphere The advantage here is that the combined problem of neutron-transport,neutron induced gamna productio and gamma transport ia done in one calculation with coupled neutron gamma cross-sectionsets Unfortunately, up until very recently, the neutron and gamma production cross sections have been prepared separately It was * therefore not surprising that we had to match up m the neutron and gamma production data accordingly This was especially true in the thermal energy range II FORMAT FOR COUPLED NEUTRON-GANNA CROSS SECTION SETS The general format of a coupled neutron-gannna cross-section set is shown in Table I The first column lists the discrete ordinate S format for n cross sections used at LASL, ie, u a f ~g ~gg u g-l%> g_2+gs s Ug_41% The table length in the vertical direction is 45 The 30 neutron and 12 gamma group numbers are labeled along the top The cross section sets in thla report do not contain any photoneutron productio and an energy upscatter mechanism for neutrons or gammas is not allowed for The neutron-energy group structure (1 through 30) is listed in Table 11 and the gamma-energy group structure is listed in Table III The multigroupmultitable cross-section sets for the 29 materials are listed in the Appendix A LASL code NGXSEC was written by one of us (Al+i)to assemble the three components for the coupled sets, namely, neutro gamma, and gamma-production cross sections 1

I TABLE I FORMAT FOR 42-GRoUP (30 NEUTRON AND 12 GANNA) COUPLED NZUTRON-GAMMA CROSS SECTION SETS IxSEC! NEUTRON GROUPS I GAMMA GROUPS I ccl Vuf 9 I 2 3 4 5 2, 2; 27 28 29 30 3! 32 33 134 35/36137138/39/40/41 42 -_w ~31-?l - Cl- I -9 rl- 3Q--!pl-32 II-2-Q 32--33!-33 %-3-g i GAMMA-TRANSPORT CROSS SECTIONS 30--31-34 @-=Q- 1$-5-9 f ~-+g b34 3-35 J~ 31- % -7-g ~-&g -9 -g -lo-g -1 l-q -12-9 -13-g -[4-g --ls-g ~-16-g NEUTRON-TRANSPO RT CROSS,SECTIONS =&17-g 30-37 31-38 53E$31-39 30-3 31-40 3w4q 3{-41 30-4! 31-42 -4?j_-18-g _?j -19-9 GAMtJA-PRODUCTION CROSS SECTIONS %-20-6 %-21-g : -22-y?J -23-g %-24-g u g-25-g u g-26-g 0 ḡ-27-g : -28-g %-29-(3 5-30-IJ ml -31 5-31+ o I-32 c g-32-g o 0,-33?j-33-g o 0 0 I-34?J-34-IJ o 0 0-0 I-35 %-35-g 0 0 0 0 0,-36 &36-g o 0-0 0 0 0 I-37 % -37-g o 0 0 0 0 0 0 I-38 %38-g c1 c1 n n n n n n t -0 1-39-g _, I -40-q -41- I i m Tooo,-in 2

1 ABLE11 ENERGY BOUNDARIES, AVERAGE ENERGY, AND ENERGY ANU LETHARGY WIDTHS AND VELOCITY FOR THE LASL/TD 30-GROUP NEUTRON STRUCTURE E 17 MeV, 1 ~/s = 1 cm/sh; 1 Shake (sh) = 1o-8 sec max Group Eg (Low Boundary) Eg AE Aug Vg (Mmls) 1 2 3 4 5 150 135 120 10 779 MeV MeV MeV MeV MeV 1573 MeV 1407 MeV 1289 MeV 1101 MeV 8705 MeV 20 15 15 20 221 MeV MeV MeV MeV MeV 13 11 12 18 25 548 519 49,6 459 48 6 7 607 368 MeV MeV 6789 MeV 4508 MeV 172 239 MeV MeV 25 50 36,1 294 8 2865 MeV 3219 MeV 815 MeV 25 248 9 2232 MeV 2510 MeV 633 MeV 25 219 10 11 1738 1353 MeV MeV 1962 MeV 1527 MeV 494 385 MeV MeV 25 25 193 171 12 823 MeV 1055 MeV 530 MeV 50 142 13 14 15 5 303 184 MeV MeV MeV 6487 MeV 3962 MeV 2363 MeV 323 197 119 MeV MeV MeV 50 50 50 111 867 679 16 17 18 19 20 21 22 23 24 25 0676 0248 912 335 1235 4540 1670 614 226 832 MeV MeV MeV MeV MeV ev ev ev ev ev 1115 MeV 0410 MeV 0150 MeV 55 MeV 2034 kev 7489 kev 2753 kev 1013 kev 0373 kev 0137 kev 1164 MeV 0428 MeV 01568 MeV 577 MeV 2115 MeV 7810 ev 2870 ev 1056 ev 388 ev 1428 ev 10 10 10 10 10 10 10 10 10 10 483 295 181 107 643 390 237 144 087 053 26 27 306 113 ev ev 50 kev 186 ev 526 ev 193 ev 10 10 032 020 28 414 ev 6839 ev 716 ev 10 012 29 30 152 0139 ev ev 2509 ev 0359 ev 262 ev 151861 ev 10 70 7 3 3

I I Group 1 (31) 2 (32) 3 (33) 4 (34) 5 (35) 6 (36) 7 (37) 8 (38) 9 (39) 10 (40) 11 (41) 12 (42) III TABLE III ENERGY BOUNDARIES FOR THE LASL/TD BASIC DATA 12-GROUP GAMMA STRUCTURE E = 10 MeV msx Eg (Low Boundary) (MeV) 90 80 70 60 50 40 30 2,0 10 5 1 01 Eg J!a!l 95 85 75 65 55 45 35 25 15 75 3 055 (:V) 10 10 10 10 10 10 10 10 10 5 4 09 A Basic Neutron Cross-Section nata References No J 1 2 3 4 5 6 7 8 9 10 11 12 Isotope l-h-l l-h-2 1-H-3 2-He-3 2-He-4 3-Li-6 3-Li-7 4-Be 5-B-1O 5-B-11 6-c 7-N Source of Data Evaluation based on work of L Stewart et al, LA-4574 (1971) Evaluation based on work of A Horsley and L Stewart, LA-3271 (1968, updated 1970) Evaluation based on work of L Stewart, LA-3270 (1965, updated 1970) Evaluation based on work of L Stewart (documentationnot available)! Evaluation based on work of L Stewart (documentationnot available) Evaluation based on AWRE data (1965) Evaluation based on AWRE data (1965) Evaluation based on work of R F Hunter, VP-3, VP-1 and VP-123 (1968-1970) Evaluation based on data from LLL Howerton Library (1966) Evaluation based on data from LLL Howerton Library (1966) Evaluation based on KAPL-UK data (1965) Evaluation based on work of P G Young and D G Foster, LASL, ENDF/B-11, VAT = 506 (1971) N 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 Isotope 8-O 11-Na 12-Mg 12-A1 14-si 17-CI 18-A 19-K 20-Ca 26-Fe 29-Cu 74-W 82-Pb 92-U-235 92-u-238 Source of Data Evaluation based on work of P G Young and D G Foster, LASL, ENDF/B-111,MAT = 1134 (1971) Evaluation based on ANRE data (1965) Evaluation based on data from LLL Howerton Library (1965) Evaluation based on old LASL/3 D-4 set (1966), and work of R E Hunter, VP-103 (1970) Evaluation based on work of M Drake, GGA, ENDF/B-11, MAT 530 (1968) Evaluation based on data from LLL Howerton Library (1965) Evaluation based on old LASL/TD-4 set (1966), and work of R E Hunter, VP-73 (1969), Evaluation based on data from LLL Howerton Library (1965) Evaluation based on AWRE data (1965) Evaluation based on old LASL/TD-4 set (1966), and work of R E Hunter, VP-103 (197~) Evaluation based on UK data (1969) Evaluation based on work of R E Eunter, vp-63 (1969) Evaluation based on AWRE data (1965) Evaluation based on work of J J Berlijn et al, LA-3527 and VP-63 (1968) Evaluation based on work of J J Berlijn et al, LA-3527 and VP-63 (1968) 94-Pu-239 Evaluation based on work of R E Hunter et al, LA-3528 and VP-63 (1968) 94-Pu-240 Evaluation based on work of R l? I!unter et al, IA-3528 and VP-63 (1968) B Basic Neutron-InducedGamma-Production Cross- Section Data References JNo Isotope 1 l-h-l 2 l-h-2 3 l-h-3 4 2-He-3 5 2-He-4 6 3-Li-6 7 3-Li-7 8 4-Be Source of Data ENDF/B-111, MAT 1148 Thermal valuea adjuated by HAS/GEH No gamma production in current act No gamma production in current act No gamma production in current set No gamma production in current set Old LASL/TD-4 evaluatio Old LASL/TD-4 evaluatio u -h; g = 19-3 h = 38, adjuate!by HAS/GEH ENDF/B-111, NAT 1154, proc by Laphan u30-h; h = 31-42, adjuated by HAS/GEH

No J 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 Isotope 5-B-1O 5-B-11 6-c 7-N 8-N 11-Na 12-Mg 13-A1 14-si I?-cl 18-A 19-K 20-Ca 26-Fe 29-CU 74-W 82-Pb 92-U-235 92-U-238 Source of Data Young-Seamen described in memo 6/8/73 No gamma production In current set Neutron cross sections taken from KAPL-UK evaluation (1965); gamma-ray spectra and multiplicities based on LASL/TD-4 memo of Stewart and Hirons (11/10/71) ENDF/B-111, MAT 1133, proc by LAPHAN- 630-h, h = 31-42 adjusted by HAS/GEIi ENDF/B-111, MAT 1134, proc by LAPHAN ENDF/B-11, NAT 51, ~3&h, h = 31-4L adjusted by NAS/GEH ENDF/B-11, MAT 52 ENDF/B-111, MAT 1135, proc by LAPHAN- u30_h, h = 31-42, adjusted by HAS/GEH ENDF/B-11, MAT 53 U30 h, h = 31-42, adjusted by HAS/GEH ENDF/B-11, MAT 54, ~30_h, h = 31-42 adjusted by HAS/GEH Nade up by HAS/GEH ENDF/B-11, MAT 55, u3&h, h = 31-42, adjusted by HAS/GEH ENDF/B-11, MAT 54 u3&h, h = 31-42, adjusted by HAS/GEH ENDF/B-11, MAT 118 u3&h, h = 31-42, adjusted by HAS/GEH Based on GRT work for neutron energies >5 MeV; at lower energies, the (y) cross section from a UK evaluation was used in conjunction with the thermal capture spectrum reported Ln ORNL-4382 Young (5/73) DNA MAT = 128, 129, 13 131, 6g_h; g = 24-3 h = 31-42, adjusted by HAS/GEH ENDF/B-111, MAT 1136, proc by LAPHAN- u30_h, h = 31-42, adjusted by HAS/GEH ENDF/B Format (Stewart and Hunter) V-III N, ~g_h; g = 23-3 h = 31-42, adjusted by HAS/GEH ENDF/B Format (Stewart and Hunter) V-III N, Ug-h; g = 20-3 h = 31-42, adjusted by HAS/GEH 94-Pu-239 Based on work of Hunter and Stewart, LA-4901; available In ENDF/B format using neutron cross sections from LA-3528; local LASL MAT # = 304 ug-h; g = 22-3 h = 31-42, adjusted by HAS/GEH 94-Pu-240 Based on work of Hunter and Stewart, LA-4901; available in ENDF/B format using neutron cross sections from LA-3528: local LASL MAT //= 305 u +; g = 24-3 h = 31-42, adjusted b; HAS/GEH c Basic Gamma Cross-Section Data All gamma transport cross sections were processed using Sandia Laboratories GAMLEG 69 (Refs 4, 5), a version with additional features of LASL S GAMLEG code, written by K D Lathrop An option in GAMLEG 69 is used to account for the annihilation radiation that results when positrons created during pair-production eventa are destroyed The creation of two annihilation gammas with an energy of 511 MeV contributes to the gamma group-to group transfer cross sections and is calculated in GAMLEG 69 The pair-productionmechanism and hence the generation of annihilation radiation occurs, of course, only when primary gammas having energies greater than the pair-production threshold energy of 1022012 MeV are present If we use a coupled neutron-gamma cross-section set in a discrete ordinate S calculatio we must n set the second entry calculated by GAMLEG 69 equal to zero for all gamma groups GAMLEG 69 inserts here u f!l,g the fluorescence cross section plus Zxu ie, two times the pair-production cross PP913,sectio If erroneously these entries are left in an S n calculatio we would create neutrons from the above interactions since the second entry in the gamma groups would be treated no differently entries in the 30 neutron groups, ban he Uf;g which will distribute fission neutrona according to the 30 Xg fission spectrum numbers ACKNOWLEDGMENTS We would like to thank Doris Dunning for the tedious job of assembling the coupled cross-section sets with the Neutron Gamma Cross _ Section code NGXSEC She also made some modifications in the code ao that the data from GAMLEG69 can be read into NGXSEC properly R J LaBauve has been helpful in the adjusting of neutron and gamma production cross sections REFERENCES 1 H A Sandmeier, S A Dupree, and G E Hanse ElectromagneticPulse and Time-Dependent Escape of Neutrons and Gamma Rays from a Nuclear Explosio Nucl Sci Eng Q, 343-352 (1972) 2 J E Campbell and H A Sandmeier, Airtransport Calculations Using the LASL-NWEF Air Flux Tape and the NWEF Computer Program--CDR, US Naval Weapons Evaluation Facility (NVEF) report 1090 (1972) 5

3 Valdoata Physics Reports, LASL interual docu- Problems by the Method of Discrete Ordinates, ments written by Dr R E Hunter at Valdoata Sandia Laboratories report SC-RR-69-739 (1969) State College, Valdosta, Georgia, while under consultant contract to LASL 5 S A Dupree and H A Sandmeier, Photon Tranaport Calculations Using the Method of Discrete 4 J H Renken and K A Adama, An Improved Ordinates, Vol II: User s Manual for GAMLEGX Capability for Solution of Photon Transport and T)TPXRAY U S Naval Weapona Evaluation Facility (NVEF) report 1035 (May-July 1969) 6

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OROU? n anew 9 OROUP 10 OROUF 11 IYROUP 12 O$IOUP 13 Onow 14 *?70M60E-01 llb66zf*oo -> O0651E01-336935 E171,?65S70E-01 -a208bbzf-ol -179 z&bf 1-145693E-01 3217310E-01 19 b9b3k o13-2 S7192E-OZ -,411 S07E-131 -,322127 L-171-22360 ZL-01-01673 a7l-nl -101096t-01 -ll?51ee-171 : :38751 OC-O1 22131 JW*O0 179017k-ol -+521 E!4E01-394649L01-2712447-01 -l?65v5t Ol -12 U59W-01-107333E-O1-863833k oz +41$ 17,0E01 153651 E 211622E*O0 2557115E 32? 313Lo O0 1727 L72E JW2->E-01 - no16nc ol -18636 RE -51377 >-01-13 VE15ZE*O0-181 Z43E -:550 wleil -134870 f* -1*09?2E 33130 ZE01-91 Wl16<-01-986 9,7r01-213215E-01-45 J275E-01-563 974E01-133690E-01-77 FEWC-01 -Om?qsc-ol -95850 *E oz -1690?OC-01,lb6607F ol -127?05E-01-79061 J7E? - II U5872--OI 2a67791E02-73262 Rf-02-617816E-02 -,174 &37t oz -603016E-02 -,*39 WIW-02 -,7647 WE-02-691 b21 E-02 312747f-02-3764 WE-02 -,246374 E-02-175 S39E-02 wow 15 OUOUP 36 ORouP 17 OROUP 11 wow lq Onoup ZO OROUP 21!7 n: 337513 E*170 230 PE*oo -314107f*oo -,207?36E l16708ebo0-755?93c-!?i -48 R5f01 -?q6 46?E-nl -15393 E-121-6313669L-02 - W,M7?f02-176?nbf-n2-109 R5PE-2 -,930389E-03 753122E-03 ~ c W2445E3O 12h6bbE*ol -1622393 -*oo -734725 L -74985 SE*O0-04z515q L -Olq?oestooo -959,02k-01 59213 VIE+1-3 b13655t-7l -?2n703t-ol -,\ 792hk-01 -, M591?t -n? O?z?<??t 2 -,146 b36f-,12 -,lo739nt-n2 - Q1o O67E-O3-73 bb67t-03 7145 bol*oo -31 W60E -127450 E*O0-503 P03k-01 -,22695 LIC01-13360 Ht-OL -,73 R903k-02-4496113k-02-262 ~IWIk-02-12770 Mk-02 - M1H391t03 -, E310M6L-O3-3949k-03-3346 Z8k-03 270871303 8: Ib7B3bE Ell -,1oo751E*o1-786183C 0213913E u1z374e01 29363 LE01-101 060E O1-534050f02 3 b151j1f-02-3+ 5? bje -02,1547116 E02 v630v t03,4 b?8?e-e,3-2998 tde-03-19 5r, ne03,1446 /E o3,1225 YJE-03-9 W3VE04 (2 1511430C01 -llu711t*ol -1 O?090E O1 2256 RIE OU -,493972 t-01 -lb6063t-01 -,741113E oz -35258 LIC L3)! -,19 WIZ2E-OZ -133041 E-OZ -90? 5JIE-03 -,t,0h231k-03 15* b,7be03-17? 1ML-03 -l10330t-03-11 S913E-0* -532377E-0* - b51121e-0+ -,3631 b9e-0+ 164263 E01-130 a50e01-115916f ol -123025C*Oi -291 a10c -,333311[ -5995E-01-651 72 SE-01-12+ 13s[01-013 W161E-01 5746 97<02 4553 R8[02-27165 he02-212?13c-02 -l?9z&?f-02 -,13162-02,7213351)F-03 -t77267f-03,4 F7666E03 -,2hh1303t-03-330 F125F-03-01uo07RE-03 -,?22215F-E13-12? 16?r03 1299177c03-020 S6hf-04 631 or6e-o6-47970 &E0+ +0441*C06-2330 MlE-04 262641 E-04 -,169337F-04 19s1,, < -q6910nt -05-16 S359C04,7206E-OS 133853E-04 -,610617E-OS -494275 E-OS OROUP 22 Onow 23 OROUP 24 OROUtI 25 OROUP 26 OROUP 27 OROW 28 1645 Q5E01 -,132273E*nl -12 S601E01-3517 +1[ -,7 J19n58f rll -,1 R17 ElE- 1-513???E-n2 -,168467C- 2 -,770 P35E 3 36 Rh3r E03-17537 he-113-977,91 E-n4-66114 re04-46 R913f,6-3n153+E-r16 1 76?7LIE-114 85 b35?e,5-5, R776E-oS 356121 E-n5 -?64R01E-r13 -,?7$3*5E-05 -,181633 E-05, 16%769<*o I -1326 *1 E*01 -,126256 t*01-3513614 t*o0-7nn259t-nl -70730 se-131 -,662! 877t-q2 -l P8837t-n2-619?q3E-133 -,? P6936F-n3-1356 J5L -03-64< 3 26t-13+,353 h87k ob 243697t 4-16 Slfi&k-nb -lll~55t -O* 6, Eb47k-os -~15197E-173-0201929E-05-1310 bok35 : 16 S015E01 -,132809E*01 lzmlzt ol -,360 bbl L -7937 Bbt-0l -?19VIE-01,761701 L-02 245762 t02 -, b93833t-03-227727 t-o3 -ln5+77t -03-498357 L-04 2370111 F-04-13213 *E-04 - I194S131L05-60 b82tit-05-407 t106e-05-238207 k-05-115759e-05 16497 &f01-1327 be C01 -l Z6WME601,3 b1011e 1 V9677E01-22362?E-01 -, IIo6106E o2 - ZU!3337E02 90+50 +2-03 -,2553 W2E03 L13BI< 4E04-38901 be-04-1 L134it, E04-8726 vbl-05 -* II fi+bl E-05-3293 zze-05 ZZ3&Otl E-05 lsoobje-05 165195C*01-132919 E01 -,127073E01-363377E no Jblnt ol -2z3b7E-01 0 R2J70bf-Od 290927 E-et -103262k-Od -,3331 7?E-03 9+060 4E0* -308722E-04,1629?bE-Ob -,67$ 609 E-OLI -32142 CE-05-17 V15E!E-05-1212 S5E-03 16463 be01-132296c01-12669 se01-362639e 803792f ol -22557W-01-827209C02-302234E02-1089,9E OZ 37 Flnn7E-03-122 z4?e-03-34517 m-04 -l13276e-ob - S2b422E-05 -zb7rwe05-1179211e-05 onoup 2? OROUP 30 OROW 31 OROUP 32 OFIOUP 33 OROIJP 34 OROUP 3s 7 lb5330c*o] -133559701-126727 E*I)1 -,362 a89e nob7n L!Enl -?26@74E-01 -,,53 b476e- 2 -,30 b221f-q2-112?95e-02 -, bln?n7e n3-1*71 E9 C-113-514345E- -,16595?E-04 -,46n516E n5-153776e-q5,8642e*o0,30775 W,11-17 122 E131 -,+76 n5+tbo0 -l15i352t -035757 PE-111-131616E-nl -48 Q071 E-112-177612L-02-65!) 953t-03 -,?37506k-r73 -n529?8t -n* -07935 nlt04 Q208*IIE -OS -739980 L-rls :,134973C02,1674 u5f-02 27 Z817E02 213251Z-02,337705E-Oa 2*3120E-ot ZL90490E-02,427854 Eoz 321666E02,254186E-02 31i4iS59E-02,557 S12E-02 399516E-02 305691 E-02 24 S133E-02 K 12

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* DEUTERIUM (H2) Neutron ID = 6, I\tomic N = 1, Table 1 OUOUP 1 anoup 2 OROUP 3 b OROUP 9 OROUP T -190691E*o0 61137 a2e Izo ZO09S7E01 P r v * -,1824E?4nO132E*O0 lb3796e-nl 127665t*o0 ;:177s6 7 L16201K*O0 437612E-01 1531?LK*OO 9193142-01 1* V5J8E 88385% 81+51 oe oi Z099b5E 136 S70E a5b5do Eol 117?94C*O0 10377 ZE*O1,13 M023C*O0?733131Z4,136752E n93093e-ol 5s979at-o I -798,? 25c-01 124130C01 144603C 294551 C*O0 112031 E 57380 ZE01 3az295f ol,218+ 23E701-031? 973 E-01 16?92EE*01 36 b026e 518756 E*o0 18987?E 843323C-01,147216E*O0 38777 se 39384 *E*O0 Onow a OnOuP \ OROUP 10 OQow 11 0RO13P 12 OROIJP 13 OROUP 14-257 bc-02 1939 n7e01,209088e 3613 S3f* ab91720e-,tl b10531e-01,22 bt7n7f oo 257297E IS8564E-01,161416c ],Z7E-05 30 f-05 Z7E-05 Z17975 Enl 240390E01 2573 3E01 21881?E OI lej737wboo 1663 Jbf 516697E 520171E 4517 d0e Ianhzbt oo 25990 beb d8b604e+o0 65ql 70E-01 1153 ZIW,1592 hmfb 16 V141t*oo 993517L01,loo of boo 13n4s9L Elo 165104 C*O0 llj32ybe*oo 2 P7144k- 1 *399 J%E01,b19nb3E ol 267? 2SL-01 3$a979L ol,5 Z12r Hf-01?6b E07k-01 3 U0946C01 37171 ue-01 368873E-01,lZ7916E-01,Z153*W-02-50 EOB o:2,9505e,oi,352593 C 69+726E 521365C*O0 35!1503E 2676 V3E Zbb86UE IWZ920E*O0,lzQznolE ol 232 be-01 127522E OJ alo OoOc05 296892C01,338z23[ 666505r 529107 EoO0 b50356e 357901 E 31 1109E OO Zb43 34E 32576 SE-01 -,* OOOOOEOS 312 39hE ol 39?243E,7 S7050C 624116 E,55 Q310E OO,485131 C 377816E zlan&sc*oo 2 Q7193E-01 OnouP 14 OROUP 16 OROUP 17 OROUP 18 131201JP19 OROUP 20 OROUP 21 -,21 OOOOE-OS 319199 E01 488 Q3?<*O0 90 i55c 697? 14E*o0 623571 be oo 538 F!WlE 707919 E110 b51613f-01 - II41OOOE-OS 2460E-05 3070 E-05 4780 E-03-4750E-05,6730 E05,336045 E~Ol 339270C01 361380 E01 342316C01,3b2z90c01 34z311E oi,1271038e*o I,160551E01 1425 $?E01 14$17W*01,1627 R7E,01 lb3095c01 17777 qk nl 156913[01 1524 J5E01 152623E*01,152555E01 IS3040E01 1379 wf*131 902251 E 5024f * 454? 50 E*O0 4533 s55-456861 F*O0 11339?f ol,452321 E i?30z31e ol z9bb41e-oz,135n754c02 0a9i13E+2 52nz59t*,418069k-01 E52663E-171 onoup 22 OROUP Z3 OIEOUP 24 0!70UP 25 OROuP 26 OROUP 27 OROuP Zn -, Z4E06 1490 C-OS,3*23 b7f ol 34231 oe*o I 1431321E nl 143080E*01 1 S2802C*OI 1521305 E01 4 S5854E,455366E 595 &22E-02,a78078E-02 - Z7907 O5,3622 30E01,142606E01 152485E01,455365E,8 EIJ716E-02-3160 E-05-3650E-oS -,e13aoe-os,342303t1,3* Z302E01 3 bz35c*ol,142959e01 14 Z9+1E01,143046 E01 152754E01 15 Z811Eb01,152907E01 4 S5106E OO,+55011E 452646 E 8769 Z7E-02 EJ534r*E-02 895065E-On -20 C-05 34?331C01 14345 be01 1534 bne ol, 65 EA86E*O0 917 E45E-02 llnnljp 2* onnup 30 OROUP 31 UR17W 32 13nuuP 33 oaoup,54 cmnup 3~,710~63c-14,34231 W*01 3612151 C61 143231W*01,15 Z754E*171 36n151t*131 1990 S9E01 653967 EIJO 461212E,@Bo888E02 631579t-02,313@ J6c-oz 3607555-01 136490 C-OZ?7@7tbC-02,60131 )E01 lb9a*oe oz Z83e13C-02 z*1319f Oa 201n47r-02 lii065?c-oz 691306 E-01,71361 *f ol,7 WL710EO1 217101 t-0< 28724 SE-OZ 3971154C OZ 3 M365E-Oa 45572 LEE-OZ 607933E-02,za7350L om 360719fOZ 297172E-02,466754C-02 377164E02 316105E-OZ OUOUP 36 onoljp 37 orow 38 OROUP 39 omoup 40 Onoup 41 OROUP 42 1183 *9E-OZ q13z06ele 1 S0735*E-OZ n91808e02,6 Z8827E-r12 b9f58be-17z 7b0966E-03 I055117E*o0 953 bl19t-rz 127977E-01 n96934t-m? 689 b94e-n2 6104 FI1E-O2 561875En7 350359E-02 475597 E-02 fl 9 b13+54c-r2 363033E-03 12 Q567C 1813 *ae-01 214163E-01,13 Q9b Mt-ol,1046 O3K-O1 041799f02 707505EOZ bl Z740E-02,541765 L-O2 b191b UE-04 173912E,476011 E01,4363 <*E01 zb20z2e-01 1920 AE-01 1536 V3E-01,12 Wbl E-01 I1l+IJLIE-01 V@38t*t-02 a81519e-02,466799 E-OU,Z44621E 887 Z08E-01 6 Z7437E-01 321659L-01 23 V2QbE-01,2z07E-01 17 L1662E01 16 N114E-01 1 S76U3E-01 152993L01 1 S0314L-01 170171 E-06 364903f 337613?E,1559E*O0 63 R2119E-01 35 W76E-01,2526114 E-01 19 bf19~e-01 158677E-01, 1338zt, F-01 l15712f-ol,i0191qe-01 91066 bf-02 206 bs6c-03 5 S7751E 557 W5E 272214E-01 14

Neutron ID = 6, Atomic N = 1, Table 2 OROIIP 1 OROU? 2 OROUP s OROuP 4 OROUP OROUP & onoup 1?03:1C01 7: * ~ 1463C-01 116s6TE on,3869422 01 1317991E,7393 WE01 7357C01 17 W+5C 104847 E*OO 570912tol 120186C*O0 2 Z2286C4 8 L19135E-01,513 Z60E01?b8138E ol 3 a i:,12 W22E*O0 23+156E 64(2559K01,247371 F01,1338 z2e01 573251 E-02 3080137E*O0,378036c Q12532E01 221061C-O1,56671 le-02 1131?6C-02-07 E5L732E-03 OnolJ* a OROUP 10 OROUP 11 OROUP 12 OROUP 13 102299C OO 770644 E,21J771?f01 66q?37E 2 -?97479c02-478706 E-02-5241 19E 2-611217E-02 ~,,190687E b11960c 911527 E-111,6665 SO< 2-5991 *5E-02 -,l12776t-ol -1351111 E-01-147838C- I -,17? 965E-nl El 1631 aoe Oo 4114 LlaEo O 1452 ME*O0 2 Y9389t-01-081@ 337E-02-187156C-01 -z42769l01-278146k01 -z91463e-01-305272t-01 1467 *8E J54*JOE 15701 oe*o O 52081 If-o: 1971 +5c02,z5f17&3E-01 356713E-01-4129 NE E-01-3354 V JE-01 0177 nlbe Lll 2126 fve-02 29 J32ZE,467676 E*O0 231850E*O0 7772E-01 -,39532 EIE-02-71t1013VE-01 -,] IE z93e*o0 -,74626 SE-01 -,?li14*5t-ol -,127066E-OJ 279291 F*O0 367569E*O0 ;1072V?E OO 631163 E02, B37555E01 l&1173c oo,15 E267C -303352 E-01 32?814C,406425E 61181?E01-132215E -021@ *311E*o0-254420E -176576 E -0273150E-01 0RO13P 1s OROUP 16 OnouP 17 oroup 18 orou? lq OROUP 20 OROUP 21 4!73166E @o 437820E*o0 674666C-01 -O?11P91CO -366299E -2 S4W15E -6063 SlE-01,925647E 625021 t*o0-136399 t *nn -579113 RC*O0-396603E*o0-7 Qc25W-01 I03191E01 307869E 10485VE *01 3 W30J2E6 -+35672E*O0-276017E,3 b0727e*o0 -z144/q E-01 0390197 fol I05288C*OI 1051 04E O1 35 J906E*O0 354211 E -?42462E*O0-261178 E -8 Z346SE-02,791145E-02 105269E o1 355692C*O0-26? 3~6E*O0-018736E-02 OnouP 22 enow 23 ORouP 24 OROUP 25 OROUP 2* OROUP 2? OROUP 20 M ln521aeool 3 S6130C -,242407C*O0 -,(12 $367E02 I05242E01 3 S*388E*n0-2421 OOE*OO -!30E@27E-02 1051 O6E*O1 356378 E Z62026E*O0 -,807713C-02 105177C*O1 105225E*OI 1 OS019E O1 355101 EOO 35+965E 355393C*O0,2421 <i?e*oo -?*2*09E*O0-241936E 08133 YOE02 -,8zQ052E-OE -81837 $2E-02 105616E*O1 355 R72C -243117 E*O0 -,5446 zoe-02 OnouP 29 WOUP 30 OROUP 31 (EROUP 32 OROUP 33 onoljp 36 OROUP 35 I05312E$01 115696 E*01 351621 E I03406E*o0-26? 262E*o0,249160C -o@11299e02 0761 M50E-02,136236E-oZ :, 1696 Q7E-02 2a1644E-02 216456t-02 J51539E OE 2832 *3 E-OC 286111 E-02 451 O]lC O2 3560 b9f02 221Q774E-02 395665E-02 599351 E02 b55174e-02 364716 E-02 303662E-02 OROUP 36 OROUP 37 OROUP 36 ORouP 39 OROUP 40 ORouP 1 onoup u J! ~o a,,~4n826e-02 i23e55l-111 1368739t+7 6 b?*68t-n2 517365E-n2 b34n31e-nz 374 bs7k-02,176363e-01 Z01576E-01,123E21E01,925420E-02 731786 Eo Z 607769E-02,52130 +t-02 457404E-02,43a6tllJE ol 37270 ue-01 20s81 Wol 1*3991 O1 111767E-01 9i E13W-02 781613E02 621345c02 6046 b0f-02 759562E-01 6140 +of-ol 150363E-01 9 Z3+55E OZ 66&3 +OE-OZ 520720E-OZ,4 Z6993E-02 3b165b E-02 3135 Jnt-02,276645 E-OZ 886068 C-01,415051 E02 _,165Q39f01-12Sbb7E-01-961954[02-77553 beoz,668562e OZ -55691 of o2 -,487807 E-02 -$331783 E02 039065 +E02 382468E-01 - W0806E-02 d 15

Neutron ID = 6, Atomic N = 1, Table 3!lRoIJP 1 OIIOUP 2 OROUP 3 orow 4 OR(JUP 9 OROUP b ono(jp 7? 134 I1OC+1 9 l11394e nl 9618 V3E01 2913 LIZC-01 3307 E01 133018C 127527E 435170c01 53? 76E01 1490 we-01 L B755E-01 137 MOC,217130E-01,] I10796EoJ -831337E-OZ Onow a OROUP 9 OROUP 10 OROUP 11 OROW \z,9195 no E-01 1359 QoE 1402 h6e-oz -12z6E-01 - I18b56C01 851990 C02 OROUP 13 2119 n2c*oo 1712C -Z3230QE-01-311636 C-01 -oz03717c-01-130n05e-ol -ST6107E-OZ onoup 16 133,7 a9e LlL7 133351 E, -28098W-01 -z23nn6t-01-137668e-01 -,777944 f-172-522353e-n2 -z99r69c112 : a - 10526 ZE OO,197756E,139072E*o0 24175 ae oo -01639 a3f-01 -,311635 E-fil - Z166Z3E-01 1!:!:! -9 b9z2st n3 393106L-OP :1:!E3A6E 235398E*O0-48904 ZE OZ,6,? 69711kol -3109 o8e-oi 016136 +E01-0145568E-02 948759k oz 161035t-01,Z29063E-01-049Q1?E-o Z 5212 Y~E-01-47461-01 -,?34717E-01,634705E-03 z?7535e-01,z707z/e01,15 MYME-01,20636 ve-02 19673 ZE 141! 892E -n9b660e-01 16128 ME -l Z5b93t* -677114 E-01 390463E-01,506302 t-0l,lm1906e-oi 128129C-03 18 Z470E 511693c-02-215 Q37z Oo -,211756 [ 0131386?E -,4 is42q E-01 b77037e01 Z630917Z-01 Z09344C*O0-138182E-01-273046E*O0 -o Z15994E*O0-798269C-01 5357E01 l15p2te*o0 z370sie-01 Onou? 15 enoup lb Onou? 17 tlroup 10 oroup 1s OROUP ZO OROUP 21 z62551e no - E19aslz E-r,2-305435 E*OO -,1737 b7e, 117887r no lb6702e*o0 5z553nc ol r 4691JZOEIJO -3449 E1E -*99997E oo -93332 ne-02 201 L193E*o0 6977 E-01 S220WC*O0-309030 E*o0 -, b5131k-01,17569 +L,342890 E-01,533152E 35 SS69E 296617E-01,16997W01 53*760 C -355069E*O0 015598 ME-01 7*5053C OZ 53 S031C*O0 355167Eoo0 14066 RC01,712633COZ 53 b8z6cbo0-3 S6259E*O0 133376E01,735226E02 OROUP 22 mow 23 Onou? 2* Onou? 25 Onou? 26 OROUP 27 onoup Zn n- n; s3b179e*oo -,3551713E* 140? 37E-nl 739779E n2 O#olJ* 29 536839C -355998 E 14c040E-01?27425E-nz a - 53*933C*O0-355663C*O0 140507E-01 72630 ZE-02 536947E*o0-35 S7JOE*O0,137 be ol 731 160E-02 - s34b67c -355993E 13 b*91f ol,73957 ee OZ 6; 53sl&7c oo -35 bm5a Eoo 136769E-01 735057E02 534534E*o0-357280E*O0 129454C-01 756191 C02 OROUP 30 OROUP 31 OROW 32 OROUP 33 OROUP 36 OROUP 3* 53$719 cf313-3 S59417C*OL7 151692E-nl 729303E-02 f 135730L-02,16136 ble-02 278117C-02,215170E-OZ 3b5966E-#z,275104E-OZ :,203m5zE02 641663E-oz 340905E-02 275261E02 a ;391316E-02 582403E02 432 b66e-02 340490 E02 279523C-02 OROUP 36 OROUP 37 OROUP 38 OROUP 39 OROUP 40 OROUP 41 OROUP 62 a 5739C-02,8277 E-IIZ 563818E-02,429939E02 345@ ZSE-02,2 S2E20E02!3 b a 9155E-02 llsmnt-nl?56468e-oz 553034C-02,433768 E-n2 356460E-n2 30 Z61W-OZ 167292E-01 177755E-01,102645E-nl 70603W-OZ 5342195 OZ 429981 E-OZ 35 W44EOZ 308 E77E-OZ o; i: 3742 ubf-01 5$ B965E-01,+74619E01 2b3297E-01 123025L-01-9693133 E-o Z 113831s-01 -w1776me-oz - I03z90E-01 670356E02-4737 Z*E-02-50321E9E oz,4 b31v7e-o Z -4*7 EI17C-OZ -312 b&o EOZ,3b617*E02 2731 we02 -+ -36 O>990E-OZ b5j3e-oz -220915E-oZ -,165510[03 2 Z37WE-02-33z?bEE-oz -135155 E-02 Innsziw oz -3030 *3E-OZ -11 Z291E-02-27t IZ0E-OZ -957495E-03-1332230E-03 O* %5794 ~lle01 2 b7499e02 16

Neutron ID = 6, Atomic N = 1, Table 4 OROUP 1 onoup z OROUP 3 OROUP OROUP 9 OROUP b OROUP 7 73831zoC-02 bl R470f-n2,6978 +3 E-111,lSIJ630f-01?936J8E01 979151E-o?,2 L2350L01 6556 ZOE-01-5697 zbf03-205303 E-01 6536E-01 45 + 630E01-330275E-01-3 F86E01 z386a7e-ol 678z710E01,366936E01 -, W7848E-01 -,246 n4qe-01-15555 ne ol -,742 bb9e-oz 1 Q64F*O0-780713 E-02-704452 C-01 -z64703e-01 737 n20c oz -01598 Q7E-02 102492E-O2 OROUPa onoup Q EIROUP 10 mow 11 oroup 12 OROUP 13 691860 C01,9691 15E OZ 33537 ae-131-636630 co z 42460 FIE-oZ 627017E-02 b2570b En2 60 E1140E-oZ 721540E01 615560E-01 5$3930c01 879658 C01 653 S96E- 1 5691E01 3913 we-01-913806 <-01 66tJ701C-01-953 Q25E-01-1059 VVE OO -,197164E -941110 L-712 -,35 R770E-01-61n35bE01 9>503ZL-01,E37241E IIz,11474 LIE01-21357 >1 C-02 53 b3n9e 3 133644 E-F1, 1225s5E-nl,211338[-01 167172 RE-01 Z96066E01 2157 *0f-01 7 ZZ316E-01 705~12E-01 1038 not-01,671377e-oz -,3718,2c oz?6!jzu2t ol 616312t-02-19 Z7Z*E02 -, 1905wIE-01-156583f-01-138675t-01-13373 ie-01-13596 JE-03 cl -o199721e02 7983?ZEL71 -,177156F -1337,0 =E,S56819E O? 1 O1686E OO I17170E*O0 638096E02-211360E-01 903n16E-ol -216120E+o0-75721 le-01 161?E*O0 01S2566C 511793E41 51 LW33C-01-191174E-01 @noi)* Iy onoup lb OROuP 17 OROW It OROUP 19 ORouP 21 El l16179c* -2 Y?959C -835 C53E01 205171!2C(70 6 W947E01 -?*3h7bE-ol -421604 E01 OROLP z? 11?318E -3761 R8t,1083 f10e*o0 20@27E,0n -3 S6*70E-111-055629 me-ol OROUP Z3 I*4860E -160541 E 177 Q83E*O0-3359116G01-2 C3622E-01 OROUP 24,14 W38E -01 E136Z6E* 652 S11E-01-15135110E41 OROUP 2s,1696 b4f -1876 WE*O0 651953E-01,63 M698E oi! OROUP Zb C805?E 150 bolc017 l 66357?F-01 60656 SC OZ OROIJP 27 149811 E*o0 -laa905e Oo 669995E-01-623232E02 OROUP 28 17 149966 C0(3-1 E7923Eoo0 667471 E-01 -,62646?E n2 ~ 16 W63E*O0-198068E*O0 665561 E- ~ -,61 EJOloE-n2 I! oomc oo -1 EJ8104E*OO 665631 E-01 -,617067f-oz 150121 E -l Eins6vEeoo 6679 cve01-6 Z06W1OZ,l*9915f oo -18 M+b7E* 66 V160E-01-626391 E-oz OROLIP Z9 OROUP 30 ORouP 31 OROUP 32 OROUP 33 OROUP 34 OROUP 35 16 Q5*IE*O0-186 z67e*o0 660225E-01-619168E-02 r 134973COZ lb74u8e-oz Z7Z877E,Z13Z51C-OZ 337705E-OZ,Z631Z6E-OZ 326 @59E-oZ 55751,?E02 399516 E-02 305691 E-o Z 205133E-02 OROUP 36 onotjp 37 Onow Ja OROUP M onoup 40 OROUP 41 OROUP 42 QZ Z80b90E-02 4 Z7LIS4E-OZ 321666E OZ Z54186f-OZ 551793 Sf O2 7 S0617E02,5nz407Eoz 367 Q89E-02 Z136S15E-OZ 23 ZQ35E-02! 13 Q W849Z[-OZ I046Z?E01 62? Q50E-02 43 L18?oC-02 3 Zl175E-r2 ZS3159E-PZ 21375 SCE-02 154095E-01 14 SZ?OCO; 7095E-02 4 Z69V3E-OZ 21391!66E-oz Z122?3E-OZ 163713E-OZ 131080E-OZ z91952e-01 1373 zee-ol 17 b36ve-oz -70 RowJE-03-15383 te-02-17t9d1e-0z -,lelo3de-02-1777 Y+E-02 - I?1460E-oz 3 Z3163E-01 - C37+13E-OZ 115033 C-01 -,abe05 E-oz -65 EWQE-04 - S36275L-04-04c +1 47E-02-3 R703 i E-01-3397 JnE-oi -30 Z637E-OZ 145791 E-01 -ol198m3e-01 058z87E-03,31253 PE-OZ 285349 E-132 2 C5571F02 212267F-OZ,1 S5E75E-02,16+ Q03E-02,147 QMFOZ 136117E-02 bs8b66e-oz -+30531 E-03 17